Korschinek, G.; Bergmaier, Andreas; Faestermann, Thomas; Gerstmann, U. C.; Knie, K.; Rugel, G.; Wallner, A.; Dillmann, I.; Dollinger, Günther; von Gostomski, Ch. L.; Kossert, K.; Maiti, M.; Poutivtsev, M.; Remmert, A.
Document type:
Zeitschriftenartikel / Journal Article
Title:
A new value for the half-life of 10Be by Heavy-Ion Elastic Recoil Detection and liquid scintillation counting
Journal:
Nuclear Instruments and Methods in Physics Research Section B
Volume:
268
Issue:
2
Year:
2010
Pages from - to:
187-191
Language:
Englisch
Keywords:
Accelerator mass spectrometry ; Accuracy and precision ; Elastic recoil detection ; Independent measurement ; Isotopic ratios ; Least square fits ; Liquid-scintillation counting ; Low energies ; Specific activity ; Spectrometric methods ; Standard errors ; Weighted mean, Cosmology ; Dosimetry ; Flowcharting ; Heavy ions ; Liquids ; Luminescence ; Mass spectrometers ; Mass spectrometry ; Particle accelerators ; Scintillation ; Scintillation counters, Radioactivity
Abstract:
The importance of 10Be in different applications of accelerator mass spectrometry (AMS) is well-known. In this context the half-life of 10Be has a crucial impact, and an accurate and precise determination of the half-life is a prerequisite for many of the applications of 10Be in cosmic-ray and earth science research. Recently, the value of the 10Be half-life has been the centre of much debate. In order to overcome uncertainties inherent in previous determinations, we introduced a new method of high accuracy and precision. An aliquot of our highly enriched 10Be master solution was serially diluted with increasing well-known masses of 9Be. We then determined the initial 10Be concentration by least square fit to the series of measurements of the resultant 10Be/9Be ratio. In order to minimize uncertainties because of mass bias which plague other low-energy mass spectrometric methods, we used for the first time Heavy-Ion Elastic Recoil Detection (HI-ERD) for the determination of the 10Be/9Be isotopic ratios, a technique which does not suffer from difficult to control mass fractionation. The specific activity of the master solution was measured by means of accurate liquid scintillation counting (LSC). The resultant combination of the 10Be concentration and activity yields a 10Be half-life of T1/2 = 1.388 ± 0.018 (1 s, 1.30 «
The importance of 10Be in different applications of accelerator mass spectrometry (AMS) is well-known. In this context the half-life of 10Be has a crucial impact, and an accurate and precise determination of the half-life is a prerequisite for many of the applications of 10Be in cosmic-ray and earth science research. Recently, the value of the 10Be half-life has been the centre of much debate. In order to overcome uncertainties inherent in previous determinations, we introduced a new method of h... »